[Terrapreta] Fw: "open-air dirt mound kiln"

joe ferguson jferguson at nc.rr.com
Wed Oct 3 09:46:09 EDT 2007


Sean K. Barry wrote:
>  
> ----- Original Message -----
> *From:* Sean K. Barry <mailto:sean.barry at juno.com>
> *To:* Robert Klein <mailto:arclein at yahoo.com>
> *Sent:* Tuesday, October 02, 2007 5:11 PM
> *Subject:* Re: [Terrapreta] "open-air dirt mound kiln"
>
> Hi Robert,
>  
> You will have to study this more carefully, I think.
>  
> As, I see it there are three possibilities with the operation of a 
> "dirt mound kiln";
>  
> 1) After and if pyrolysis commences, appropriately limiting the oxygen 
> intake and "producer gas" with an H2, CO, CO2, N2, and CH4 content 
> close to what I predicted will vent, unburned, from the kiln to the 
> atmosphere (no flames).  This may leave maybe 25% of the dry biomass 
> weight in charcoal/ash (~40% by volume).  The rest of the matter from 
> the biomass WILL vent to the atmosphere as "producer gas".  Unless it 
> is capture and burned in a flame (a "flare"), then it will go 
> unchanged into the atmosphere, and very fast!  Free hydrogen gas at 
> atmospheric pressure and temperature has a buoyancy such that it rises 
> at 17,000 miles per hour from the surface.  This is faster than escape 
> velocity.
Where on earth did you get that number? URL, please?
> The emissions gases are "hot".
>  
> 2) Enough oxygen will enter the dirt mound and most of the biomass 
> carbohydrates will completely combust and vent to the atmosphere as 
> CO2 and H2O, leaving little or no charcoal and the rest as white ash.
>  
> 3) The oxygen intake is so limited that the "burn" quenches before 
> pyrolysis begins, leaving some combusted biomass and some raw 
> un-combusted biomass.  Most of the exhaust will be CO2, H2O and carbon 
> soot (smoke).  The pyrolysis reaction can be quenched too, but this 
> would mean that the flow of oxygen into the mound kiln would almost 
> have to be completely blocked.
>  
> You may not agree with any of this analysis.  Hopefully, if you ever 
> try this and want to have it adopted on a large scale by other people, 
> then you will figure out a way to measure the emissions from this 
> "dirt mound kiln".
>  
> My stated opinion now, still, and before is that The efficiency of a 
> "dirt mound charcoal kiln" (charcoal mass/feedstock mass) will be low 
> and it will vent significant GHG in operation, if it can be made to 
> work at all.
>  
> Richard Haard and Larry Williams tried this (on the 'terrapreta' 
> list).  They did not know what I have been trying to tell you when 
> they did it, either.  They had some trouble making it work, although 
> they finally were able to produce some charcoal.  Clean (in the 
> limited or no potent GHG sense), efficient pyrolysis of biomass IS NOT 
> EASY.  It is certainly not as easy as piling up corn stalks under root 
> balls and lighting it on fire.
>  
> Regards,
>  
> SKB
>
>     ----- Original Message -----
>     *From:* Robert Klein <mailto:arclein at yahoo.com>
>     *To:* Sean K. Barry <mailto:sean.barry at juno.com>
>     *Sent:* Tuesday, October 02, 2007 4:08 PM
>     *Subject:* Re: [Terrapreta] Biochar Packing Strategies
>
>     Hi Sean
>
>     I will add one quick comment at the moment.  The
>     earthen kiln that is constructed would be a closed
>     shell including a topping of dirt.  This will tend to
>     naturally grab the heavies coming off the hot zone.
>     And the operator would stand by to throw dirt on any
>     breakthroughs.
>
>     As you also pointed out, the shell is naturally leaky
>     to gases, including oxygen.  Thus it is reasonable to
>     suppose that there is a steady but slow supply of
>     oxygen which sustains the burn.
>
>     I suggested that the burn is initiated through the
>     expedient of emptying a bowl of red hot wood coals on
>     the top of the stack,  tipping the bowl on top of the
>     burn and covering same with mud.  This prevents the
>     burning charge from been stifled as the charge
>     migrates to the bottom of the stack.
>
>     This hot spot will draw in oxygen through the stack
>     and  force production gas into the walls of the
>     glowing chimney been created.
>
>     Now I want to talk about the stoichiometry of the
>     production gases.  The gases will burn preferentially
>     with the hydrogen and methane burning first,
>     especially since they are been produced at a high
>     temperature as you pointed out.
>
>     This means that the methane and hydrogen end will be
>     substantially reduced throughout the burn.  The dirt
>     shell helps a second time by slowing the exit of the
>     gases.
>
>     And yes there will still be leakage.
>
>     Field trials can resolve the actual numbers relating
>     to a well managed biochar burn.  At this point,
>     though, I suggest that light flammable gases will be
>     much less than anyone imagined.
>
>     By the way,has anyone determined the methane
>     production of a smoldering forest floor that is the
>     result of a forest fire or a slash and burn operation?
>      It will clearly be at least equivalent to the
>     carefully controlled earthen kiln as described.  Such
>     a global calculation will actually give us an upper
>     limit to the  amount of gases we want to permit
>     globally since this method can replace and eventually
>     displace slash and burn.
>
>     regards
>
>     Bob
>
>
>     --- "Sean K. Barry" <sean.barry at juno.com
>     <mailto:sean.barry at juno.com>> wrote:
>
>     > Hi Robert,
>     >
>     > The pyrolysis reaction (otherwise known as
>     > destructive distillation and/or partial combustion)
>     > of biomass in air as the oxidant, generates
>     > "producer gas".  "Producer gas" is a mixture of
>     > exhaust gases from complete combustion; Carbon
>     > dioxide gas-CO2 and Water as a gas-H2O, un-reacted
>     > inert gases; Nitrogen gas-N2, and some energy
>     > containing fuel gases; Hydrogen gas-H2, Carbon
>     > monoxide gas-CO, and Methane gas-CH4.  There are
>     > also some longer string hydrocarbons (e.g. Ethane
>     > gas-C2H4, etc.) and some vaporized tars (these are
>     > even longer string hydrocarbons and/or aromatic
>     > hydrocarbons, consisting partly of 6-carbon benzene
>     > rings and parts of benzene rings) in very small
>     > amounts (15-2000 ppm).  There can be un-reacted
>     > Oxygen-O2, too, if the reaction has been quenched
>     > (dropped below the ignition temperature of the
>     > biomass feedstock and the other gases).
>     >
>     > The "producer gas" is not generated in any large
>     > volume until most of the water is driven out of the
>     > feedstock and the temperature of the biomass exceeds
>     > about 250 degrees C, when the pyrolysis reaction
>     > begins in earnest.  The reaction requires an input
>     > of external heat (or enough input of oxygen to keep
>     > combustion occurring in the feedstock) until the
>     > temperature exceeds about 400 degrees C, when the
>     > reaction becomes exothermic and generates enough
>     > heat on its own, to continue without external energy
>     > being supplied.  Reducing the supply of oxygen to
>     > the reaction STOPS the combustion of fuel gases and
>     > thus increases the output volume of the fuel content
>     > of the "producer gas".
>     >
>     > In an "open-air" kiln, a dirt mound with biomass
>     > inside of it, there must be a supply of oxidant (the
>     > air) until the reaction becomes exothermic.
>     > Otherwise the "burn" will smolder out.  During this
>     > part of the process, Water as gas-H2O, Carbon
>     > dioxide gas-CO2, and soot (exploded off particles of
>     > carbon) will be the bulk of the output volume of the
>     > exhaust.  The feedstock will be is in a state "full
>     > combustion".
>     >
>     > The atomic weight of Hydrogen gas-H2 molecules   is
>     > 1+1 = 2, ~10-20% by volume of producer gas
>     > The atomic weight of Carbon monoxide gas-CO
>     > molecules is  12+16 = 28, ~10-20% by volume of
>     > producer gas
>     > The atomic weight of Carbon dioxide gas-CO2
>     > molecules is 12+16+16 = 44, ~10-25% by volume of
>     > producer gas
>     > The atomic weight of Nitrogen gas-N2 molecules is
>     > 14+14 = 28, ~40-50% by volume of producer gas
>     > The atomic weight of Methane gas-CH4 molecules is
>     > 12+1+1+1+1 = 16, ~2-4% by volume of producer gas
>     >
>     > Hydrogen-H2 is the lightest and Methane-CH4 is the
>     > second lightest of these gaseous components.  Only
>     > if the oxygen is limited and there is not complete
>     > combustion will there be any fuel gases left from
>     > the reaction.  There has to be flame to burn the
>     > fuel gases.  If there is no flame, then the fuel gas
>     > components will rise out of the pyrolyzing biomass
>     > and emit right into the open atmosphere.
>     > This is a measurable fact, not a hypothesis.
>     >
>     > >At the time I made any such comment, this was a
>     > very
>     > >sleepy group and you had not weighed in.  And you
>     > are
>     > >still the only person who has chosen to not agree
>     > so
>     > >far.
>     >
>     > This is not true, Robert.  Adriana Downy at BEST,
>     > Tom Miles, and Michael Bailes, have all voiced the
>     > same opinion as me about Methane-CH4 from a
>     > pyrolysis reaction.  They said it in response to you
>     > too.  Do you need for me to produce those postings?
>     > I know Stephen Joseph at BEST and Danny Day at
>     > Eprida would agree with me on this too.  Tom Reed
>     > and Aqua Das at the Biomass Energy Foundation, Dr.
>     > Michael ANtal, Jr. at the University of Hawaii have
>     > all discussed this in their very close work with
>     > biomass gasification and biomass-to-charcoal
>     > reactions.  I have read from ALL of these peoples
>     > work.  They and the others on this list who really
>     > understand what a pyrolysis reaction in biomass is
>     > know that what I am saying is true.  Methane-CH4
>     > emissions from a pyrolysis reaction at only 2-4%
>     > levels are still potent GHG contributers.
>     >
>     > Just because some do not respond to you does not
>     > constitute agreement with you.  Just because you
>     > miss or ignore the contradictory responses does not
>     > constitute agreement with you.  I am not a member of
>     > the "sleepy" part of this group.  I am not
>     > disagreeing with you based on just being contrary.
>     > I am arguing a valid point with you.  I disagree
>     > firmly and I can back up what I say about it.  You
>     > can't believe I think it is fair for you to go to
>     > your blog and say I and everyone else here on the
>     > 'terrapreta' list agrees with you.
>     >
>     > Robert, the troposphere is the lowest part of the
>     > atmosphere.  Methane-CH4 concentrations in the
>     > atmosphere from the troposphere all the way up
>     > through the stratosphere and ionosphere are rising
>     > and have been rising for some time.  Methane-CH4 is
>     > decomposed in the atmosphere by reactions with
>     > oxygen, just like combustion.  The half-life of
>     > Methane-CH4 in the atmosphere is ~ 7 years.  That
>     > means it takes ~7 years for only half of the
>     > Methane-CH4 to decompose.  It does not all decompose
>     > within 7 years.  Methane-CH4 has a much greater
>     > ability to absorb and reflect infrared radiation
>     > shooting up from the Earth's surface, than
>     > Carbon-dioxide does.
>     >
>     > Natural gas is predominantly Methane gas-CH4, some
>     > Carbon monoxide gas-CO, and some Hydrogen gas-H2.
>     > When we burn it, those fuels are "fully combusted"
>     > in flames (that is evidence of the exothermic nature
>     > of combustion) and the fuel gases are gone,
>     > converted into exhaust gases, CO2 and H2O.  That is
>     > also accepted chemistry and a measurable fact.  I
>     > have told you that Methane-CH4 emissions from a
>     > pyrolysis reaction can be "flared".  That means
>     > burning them.  No flames means emission of the
>     > un-burned gases, including Methane-CH4.  It is that
>     > simple.
>     >
>     > I suggested to you that you could read
>     >
>     http://en.wikipedia.org/wiki/Methane<http://en.wikipedia.org/wiki/Methane
>     <http://en.wikipedia.org/wiki/Methane%3Chttp://en.wikipedia.org/wiki/Methane>>
>     > and
>     >
>     http://en.wikipedia.org/wiki/Green_house_gas<http://en.wikipedia.org/wiki/Green_house_gas
>     <http://en.wikipedia.org/wiki/Green_house_gas%3Chttp://en.wikipedia.org/wiki/Green_house_gas>>
>     > to get a better understanding of what I am reporting
>     > to you.  I do not believe that I am contradicting
>     > anything that is said there.  Those pages are
>     > correct information, that is widely accepted and is
>     > documented in several other reputable sources.
>     >
>     > Look here->
>     >
>     http://en.wikipedia.org/wiki/Global_warming_controversy<http://en.wikipedia.org/wiki/Global_warming_controversy
>     <http://en.wikipedia.org/wiki/Global_warming_controversy%3Chttp://en.wikipedia.org/wiki/Global_warming_controversy>>
>     > ...
>     > Look here->
>     >
>     http://en.wikipedia.org/wiki/Climate_change_denial<http://en.wikipedia.org/wiki/Climate_change_denial
>     <http://en.wikipedia.org/wiki/Climate_change_denial%3Chttp://en.wikipedia.org/wiki/Climate_change_denial>>
>     > for even more information.
>     >
>     > This is an important issue to me, Robert.  You can
>     > dismiss it, if you want to.  You sure seem to want
>     > to.  But, please DO NOT associate your views with
>     > agreement from me anymore.
>     >
>     > Please note that I am not brow beating you in front
>     > of the rest of this group.  I want to, but I am not
>     > doing it, because some of them get their panties in
>     > a bunch over reading ti, thinking that I need to not
>     > argue so vigorously with you anymore.  You keep
>     > coming back to me with claims that my views are
>     > remarkable assertions and imply that they are just
>     > opinions or unwarranted.  I do present valid support
>     > for what I say.  Go ahead and read some of it.  You
>     > do not discuss this in scientific terms with me and
>     > you do not rebut effectively anything I say.
>     >
>     > I appreciate any interest or traffic that you can
>     > bring to the 'terrpreta' list.  But, would you
>     > please give me some level of respect by not saying
>     > agreements with you were made with ALL of the
>     > members on this list and then go post that to your
>     > blog anymore?
>     >
>     >
>     > Regards,
>     >
>     > SKB
>     >   ----- Original Message -----
>     >   From: Robert Klein<mailto:arclein at yahoo.com>
>     >   To: Sean K. Barry<mailto:sean.barry at juno.com>
>     >   Sent: Monday, October 01, 2007 5:47 PM
>     >   Subject: Re: [Terrapreta] Biochar Packing
>     > Strategies
>     >
>     >
>     >
>     >   Hi Sean
>     >
>     >   Let us reply line by line to your concerns.
>     >
>     >   --- "Sean K. Barry"
>     > <sean.barry at juno.com<mailto:sean.barry at juno.com
>     <mailto:sean.barry at juno.com%3Cmailto:sean.barry at juno.com>>>
>     > wrote:
>     >
>     >   > Robert,
>     >   >
>     >   > Everything you say is conjecture.  For you to
>     > say
>     >
>     === message truncated ===
>
>
>
>           
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